APL Materials (Jan 2020)

Magnetic exchange induced Weyl state in a semimetal EuCd2Sb2

  • Hao Su,
  • Benchao Gong,
  • Wujun Shi,
  • Haifeng Yang,
  • Hongyuan Wang,
  • Wei Xia,
  • Zhenhai Yu,
  • Peng-Jie Guo,
  • Jinhua Wang,
  • Linchao Ding,
  • Liangcai Xu,
  • Xiaokang Li,
  • Xia Wang,
  • Zhiqiang Zou,
  • Na Yu,
  • Zengwei Zhu,
  • Yulin Chen,
  • Zhongkai Liu,
  • Kai Liu,
  • Gang Li,
  • Yanfeng Guo

DOI
https://doi.org/10.1063/1.5129467
Journal volume & issue
Vol. 8, no. 1
pp. 011109 – 011109-8

Abstract

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Magnetic Weyl semimetals (WSMs) bearing long-time seeking are still very rare. We have identified herein that EuCd2Sb2, a semimetal belonging to the type IV magnetic space group, hosts a magnetic exchange induced Weyl state via performing high magnetic field magnetotransport measurements and ab initio calculations. In the A-type antiferromagnetic structure, the external field larger than 3.2 T can align all Eu spins to be fully polarized along the c-axis and consequently drive EuCd2Sb2 into a spin polarized state. Magnetotransport measurements up to ∼55–60 T showed striking Shubnikov-de Hass oscillations associated with a nontrivial Berry phase. The ab initio calculations unveiled a phase transition of EuCd2Sb2 from a small gap antiferromagnetic topological insulator to a spin polarized WSM in which the Weyl points emerge along the Γ-Z path. Fermi arcs on (100) and (010) surfaces are also predicted. Meanwhile, the observed large anomalous Hall effect indicates the existence of Weyl points around the Fermi level. The results pave a way toward the realization of various topological states in a single material through the magnetic exchange manipulation.