Drivers of a Summertime Combined High Air Pollution Event of Ozone and PM_2.5 in Taiyuan, China

Abstract

Combined air pollution of ozone and PM2.5 often occurs in coal-based cities of China such as Taiyuan City. In this study, the Weather Research and Forecasting/Chemistry (WRF-Chem) model was employed to simulate a combined high air pollution event of ozone and PM2.5 in Taiyuan City from 20 May to 29 May 2015,with the maximum daily 8-hour average (MDA8) for ozone exceeding 140 ppbv and PM2.5 concentrations surpassing 200µgm−3. We further investigated the drivers of the combined air pollution in Taiyuan during the polluted period. The simulation results showed that the model can well simulate the combined pollution event in Taiyuan, with assessment parameters within reasonable ranges. Moreover, by analyzing the observational data and simulations, the major factors causing the PM2.5 pollution in Taiyuan during this time period were suggested to be local emissions and pollutant transport from the North China Plain (NCP) located to the east of Taiyuan. In addition, unfavorable meteorological and geographical conditions in Taiyuan also play important roles in forming severe PM2.5 pollution. Regarding the ozone pollution in Taiyuan, we suggest that the mechanism dominating the pollution event is that of ozone-rich air being transported to Taiyuan at high altitudes and then mixed downwards, resulting in an increase of the ground-level ozone in Taiyuan. Furthermore, we found local emissions and emissions from Taiyuan Basin and Henan Province, which are located to the south of Taiyuan, contributing significantly to the ozone pollution in Taiyuan City during this time.

Keywords

• ozone
• PM_2.5
• combined high pollution
• Taiyuan
• air quality