Anion-enrichment interface enables high-voltage anode-free lithium metal batteries

Minglei Mao; Xiao Ji; Qiyu Wang; Zejing Lin; Meiying Li; Tao Liu; Chengliang Wang; Yong-Sheng Hu; Hong Li; Xuejie Huang; Liquan Chen; Liumin Suo

doi:10.1038/s41467-023-36853-x

Nature Communications (Feb 2023)

Anion-enrichment interface enables high-voltage anode-free lithium metal batteries

Minglei Mao,
Xiao Ji,
Qiyu Wang,
Zejing Lin,
Meiying Li,
Tao Liu,
Chengliang Wang,
Yong-Sheng Hu,
Hong Li,
Xuejie Huang,
Liquan Chen,
Liumin Suo

Affiliations

Minglei Mao: Beijing Advanced Innovation Center for Materials Genome Engineering, Institute of Physics, Chinese Academy of Sciences, Beijing National Laboratory for Condensed Matter Physics
Xiao Ji: School of Integrated Circuits, School of Optical and Electronic Information, Wuhan National Laboratory for Optoelectronics (WNLO), Optics Valley Laboratory, Huazhong University of Science and Technology
Qiyu Wang: Beijing Advanced Innovation Center for Materials Genome Engineering, Institute of Physics, Chinese Academy of Sciences, Beijing National Laboratory for Condensed Matter Physics
Zejing Lin: Beijing Advanced Innovation Center for Materials Genome Engineering, Institute of Physics, Chinese Academy of Sciences, Beijing National Laboratory for Condensed Matter Physics
Meiying Li: Beijing Advanced Innovation Center for Materials Genome Engineering, Institute of Physics, Chinese Academy of Sciences, Beijing National Laboratory for Condensed Matter Physics
Tao Liu: Beijing Advanced Innovation Center for Materials Genome Engineering, Institute of Physics, Chinese Academy of Sciences, Beijing National Laboratory for Condensed Matter Physics
Chengliang Wang: School of Integrated Circuits, School of Optical and Electronic Information, Wuhan National Laboratory for Optoelectronics (WNLO), Optics Valley Laboratory, Huazhong University of Science and Technology
Yong-Sheng Hu: Beijing Advanced Innovation Center for Materials Genome Engineering, Institute of Physics, Chinese Academy of Sciences, Beijing National Laboratory for Condensed Matter Physics
Hong Li: Beijing Advanced Innovation Center for Materials Genome Engineering, Institute of Physics, Chinese Academy of Sciences, Beijing National Laboratory for Condensed Matter Physics
Xuejie Huang: Beijing Advanced Innovation Center for Materials Genome Engineering, Institute of Physics, Chinese Academy of Sciences, Beijing National Laboratory for Condensed Matter Physics
Liquan Chen: Beijing Advanced Innovation Center for Materials Genome Engineering, Institute of Physics, Chinese Academy of Sciences, Beijing National Laboratory for Condensed Matter Physics
Liumin Suo: Beijing Advanced Innovation Center for Materials Genome Engineering, Institute of Physics, Chinese Academy of Sciences, Beijing National Laboratory for Condensed Matter Physics

DOI: https://doi.org/10.1038/s41467-023-36853-x
Journal volume & issue: Vol. 14, no. 1
pp. 1 – 13

Abstract

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The implementation of Li metal anode with high-voltage Ni/Co rich cathode is plagued by low coulombic efficiency and inferior cycling stability. Here authors propose an anion-enriched interface to facilitate the columnar-structure of Li deposits to solve this issue.

Published in Nature Communications

ISSN: 2041-1723 (Online)
Publisher: Nature Portfolio
Country of publisher: United Kingdom
LCC subjects: Science
Website: https://www.nature.com/ncomms/

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