High-Order Harmonic Generation in Au Nanoparticle-Contained Plasmas
Mottamchetty Venkatesh,
Rashid A. Ganeev,
Dmitry S. Ivanov,
Ganjaboy S. Boltaev,
Vyacheslav V. Kim,
Jingguang Liang,
Andrey A. Samokhvalov,
Andrei V. Kabashin,
Sergey M. Klimentov,
Martin E. Garcia,
Chunlei Guo
Affiliations
Mottamchetty Venkatesh
The Guo Photonics Laboratory, State Key Laboratory of Applied Optics, Changchun Institute of Optics, Fine Mechanics and Physics, Chinese Academy of Sciences, Changchun 130033, China
Rashid A. Ganeev
The Guo Photonics Laboratory, State Key Laboratory of Applied Optics, Changchun Institute of Optics, Fine Mechanics and Physics, Chinese Academy of Sciences, Changchun 130033, China
Dmitry S. Ivanov
Institute of Physics and Center for Interdisciplinary Nanostructure Science and Technology (CINSaT), University of Kassel, 34125 Kassel, Germany
Ganjaboy S. Boltaev
The Guo Photonics Laboratory, State Key Laboratory of Applied Optics, Changchun Institute of Optics, Fine Mechanics and Physics, Chinese Academy of Sciences, Changchun 130033, China
Vyacheslav V. Kim
The Guo Photonics Laboratory, State Key Laboratory of Applied Optics, Changchun Institute of Optics, Fine Mechanics and Physics, Chinese Academy of Sciences, Changchun 130033, China
Jingguang Liang
The Guo Photonics Laboratory, State Key Laboratory of Applied Optics, Changchun Institute of Optics, Fine Mechanics and Physics, Chinese Academy of Sciences, Changchun 130033, China
Andrey A. Samokhvalov
Department of Laser Photonics and optoelectronics, ITMO University, 197101 St. Petersburg, Russia
Andrei V. Kabashin
National Research Nuclear University MEPhI (Moscow Engineering Physics Institute), 115409 Moscow, Russia
Sergey M. Klimentov
National Research Nuclear University MEPhI (Moscow Engineering Physics Institute), 115409 Moscow, Russia
Martin E. Garcia
Institute of Physics and Center for Interdisciplinary Nanostructure Science and Technology (CINSaT), University of Kassel, 34125 Kassel, Germany
Chunlei Guo
The Guo Photonics Laboratory, State Key Laboratory of Applied Optics, Changchun Institute of Optics, Fine Mechanics and Physics, Chinese Academy of Sciences, Changchun 130033, China
Gold nanoparticles (NPs) have a wide range of applications in various fields. Here, we present high-order nonlinear optical studies of the plasmas produced from ablation of Au bulk targets and Au NP films deposited on paper and glass substrates. Experimentally, we analyze high-order harmonic generation (HHG) from gold NPs-containing plasmas. The HHG is produced by 35-fs pulses at 800 and 400 nm, while the plasmas are produced by femtosecond (35 fs, 800 nm), picosecond (200 ps, 800 nm), and nanosecond (5 ns, 1064 nm) pulses, respectively. High-order harmonics produced from ablated Au NPs on paper were 40 times stronger than the HHG from that ablated from the Au bulk targets. Through molecular dynamic simulations, we investigate the formation of gold NPs during laser ablation of a metal surface under different conditions.