EPJ Web of Conferences (Jan 2019)

Vibrational Interferometry Enables Single-Scan Acquisition of all χ(3) Multi-Dimensional Coherent Spectra

  • Travis M. Autry,
  • Moody Galan,
  • McDonald Corry,
  • James M. Fraser,
  • Richard P. Mirin,
  • Kevin L. Silverman

DOI
https://doi.org/10.1051/epjconf/201920503013
Journal volume & issue
Vol. 205
p. 03013

Abstract

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We demonstrate a new method for multidimensional coherent spectroscopy of nanostructures. We use a heterodyne technique implemented with a confocal microscope to record the amplitude and phase of all degenerate third-order wave-mixing processes.