Scientific Reports (Jan 2024)
Colossal Kerr nonlinearity without absorption in a five-level atomic medium
Abstract
Abstract In this work, we present an analytical method to achieve giant Kerr nonlinearity without absorption in a five-level atomic medium. By using iterative perturbation technique on density matrix equations, we have derived the analytical expressions of nonlinear susceptibility and Kerr nonlinear coefficient in the presence of spontaneously generated coherence (SGC) and relative phase between applied laser fields. It shows that, this five-level atomic medium exhibits multiple electromagnetically induced transparency (EIT) at three different frequencies, at the same time, the Kerr nonlinear coefficient is enhanced around three transparent spectral regions; in each such EIT region appears a pair of positive–negative peaks of Kerr nonlinear coefficient. In particular, these nonlinear peaks are moved to the center of the EIT windows via SGC. This means that the Kerr nonlinear coefficient is enhanced with completely suppressed absorption at different transparency frequencies. Furthermore, the magnitude and the sign of the Kerr nonlinear coefficient are easily controlled according to the SGC strength, the coupling laser intensity, and the relative phase between applied laser fields. Such a giant nonlinear medium can be useful for photonic devices working in the resonant frequency region without absorption. As a typical application, this giant Kerr nonlinear material has been applied to an interferometer for the formation of optical bistability, and showed the appearance of OB at the resonant frequency with significantly reduced threshold intensity and OB width.