Giant (Mar 2022)
Chiral 1D perovskite microwire arrays for circularly polarized light detection
Abstract
Detection of circularly polarized light (CPL) accelerates the development of various optical technologies, but the additional quarter-wave plate and linear polarizer are required for conventional polarized light detectors, resulting in tremendous difficulty in integration and miniaturization of the devices. Herein, we fabricate pure (010)-orientated chiral one-dimensional (1D) perovskite microwire arrays with high crystallinity, strict alignment, and homogeneous size by a capillary-bridge-manipulated method. By the synergy of the excellent crystallinity and pure crystallographic orientation, high-performance CPL photodetectors are fabricated, with a maximum anisotropy factor of 0.23, responsivity exceeding 26 mA W −1, and detectivity exceeding 2.2 × 1011 Jones. Furthermore, the CPL photodetectors based on microwire arrays also exhibit impressive environmental stability under ambient conditions.