Physical Review Research (Aug 2023)

Spin injection in the doped bad metal SrTiO_{3}

  • Patrizio Graziosi,
  • Ilaria Bergenti,
  • Lorenzo Vistoli,
  • Fabio Galassi,
  • Marco Calbucci,
  • Alberto Riminucci,
  • Francesco Borgatti,
  • Donald A. MacLaren,
  • Kerry J. O’Shea,
  • Giovanni Vinai,
  • Piero Torelli,
  • Giancarlo Panaccione,
  • Viktor Kabanov,
  • Valentin Alek Dediu

DOI
https://doi.org/10.1103/PhysRevResearch.5.033096
Journal volume & issue
Vol. 5, no. 3
p. 033096

Abstract

Read online Read online

In this paper, we demonstrate the capability to establish spin-polarized currents in doped SrTiO_{3} (STO). The results are based on the study of charge and spin transport in STO layers doped by the reversible electromigration of oxygen atoms in resistive-switching La_{0.7}Sr_{0.3}MnO_{3}/STO/Co vertical stacks. The formation of oxygen vacancies inside STO results in a metallic conductivity at temperatures <200–250 K, above which a transition to an insulatinglike behavior is detected. A detailed theoretical analysis shows that the behavior of the metallic phase in our samples corresponds to the well-known state of the thermodynamically doped STO featuring the so-called bad metal behavior. Thus, our findings introduce this class of unconventional materials as valuable candidates for innovative spintronic devices.