Light: Science & Applications (Jan 2024)

Highly efficient and aberration-free off-plane grating spectrometer and monochromator for EUV—soft X-ray applications

  • Jie Li,
  • Kui Li,
  • Xiaoshi Zhang,
  • Dimitar Popmintchev,
  • Hao Xu,
  • Yutong Wang,
  • Ruixuan Li,
  • Guangyin Zhang,
  • Jiyue Tang,
  • Jin Niu,
  • Yongjun Ma,
  • Runyu Meng,
  • Changjun Ke,
  • Jisi Qiu,
  • Yunfeng Ma,
  • Tenio Popmintchev,
  • Zhongwei Fan

DOI
https://doi.org/10.1038/s41377-023-01342-9
Journal volume & issue
Vol. 13, no. 1
pp. 1 – 12

Abstract

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Abstract We demonstrate a novel flat-field, dual-optic imaging EUV—soft X-ray spectrometer and monochromator that attains an unprecedented throughput efficiency exceeding 60% by design, along with a superb spectral resolution of λ/Δλ > 200 accomplished without employing variable line spacing gratings. Exploiting the benefits of the conical diffraction geometry, the optical system is globally optimized in multidimensional parameter space to guarantee optimal imaging performance over a broad spectral range while maintaining circular and elliptical polarization states at the first, second, and third diffraction orders. Moreover, our analysis indicates minimal temporal dispersion, with pulse broadening confined within 80 fs tail-to-tail and an FWHM value of 29 fs, which enables ultrafast spectroscopic and pump-probe studies with femtosecond accuracy. Furthermore, the spectrometer can be effortlessly transformed into a monochromator spanning the EUV—soft X-ray spectral region using a single grating with an aberration-free spatial profile. Such capability allows coherent diffractive imaging applications to be conducted with highly monochromatic light in a broad spectral range and extended to the soft X-ray region with minimal photon loss, thus facilitating state-of-the-art imaging of intricate nano- and bio-systems, with a significantly enhanced spatiotemporal resolution, down to the nanometer–femtosecond level.