Nature Communications (Jan 2023)
Bottom-up evolution of perovskite clusters into high-activity rhodium nanoparticles toward alkaline hydrogen evolution
- Gaoxin Lin,
- Zhuang Zhang,
- Qiangjian Ju,
- Tong Wu,
- Carlo U. Segre,
- Wei Chen,
- Hongru Peng,
- Hui Zhang,
- Qiunan Liu,
- Zhi Liu,
- Yifan Zhang,
- Shuyi Kong,
- Yuanlv Mao,
- Wei Zhao,
- Kazu Suenaga,
- Fuqiang Huang,
- Jiacheng Wang
Affiliations
- Gaoxin Lin
- State Key Lab of High Performance Ceramics and Superfine microstructure, Shanghai Institute of Ceramics, Chinese Academy of Sciences
- Zhuang Zhang
- State Key Lab of High Performance Ceramics and Superfine microstructure, Shanghai Institute of Ceramics, Chinese Academy of Sciences
- Qiangjian Ju
- State Key Lab of High Performance Ceramics and Superfine microstructure, Shanghai Institute of Ceramics, Chinese Academy of Sciences
- Tong Wu
- State Key Lab of High Performance Ceramics and Superfine microstructure, Shanghai Institute of Ceramics, Chinese Academy of Sciences
- Carlo U. Segre
- Department of Physics & Center for Synchrotron Radiation Research and Instrumentation, Illinois Institute of Technology
- Wei Chen
- Department of Mechanical, Materials and Aerospace Engineering, Illinois Institute of Technology
- Hongru Peng
- School of Physical Science and Technology, ShanghaiTech University
- Hui Zhang
- State Key Laboratory of Functional Materials for Informatics, Shanghai Institute of Microsystem and Information Technology, Chinese Academy of Sciences
- Qiunan Liu
- SANKEN, Osaka University
- Zhi Liu
- School of Physical Science and Technology, ShanghaiTech University
- Yifan Zhang
- State Key Lab of High Performance Ceramics and Superfine microstructure, Shanghai Institute of Ceramics, Chinese Academy of Sciences
- Shuyi Kong
- State Key Lab of High Performance Ceramics and Superfine microstructure, Shanghai Institute of Ceramics, Chinese Academy of Sciences
- Yuanlv Mao
- State Key Lab of High Performance Ceramics and Superfine microstructure, Shanghai Institute of Ceramics, Chinese Academy of Sciences
- Wei Zhao
- State Key Lab of High Performance Ceramics and Superfine microstructure, Shanghai Institute of Ceramics, Chinese Academy of Sciences
- Kazu Suenaga
- SANKEN, Osaka University
- Fuqiang Huang
- State Key Lab of High Performance Ceramics and Superfine microstructure, Shanghai Institute of Ceramics, Chinese Academy of Sciences
- Jiacheng Wang
- State Key Lab of High Performance Ceramics and Superfine microstructure, Shanghai Institute of Ceramics, Chinese Academy of Sciences
- DOI
- https://doi.org/10.1038/s41467-023-35783-y
- Journal volume & issue
-
Vol. 14,
no. 1
pp. 1 – 10
Abstract
Self-reconstruction is an efficient method to synthesize active electrocatalysts. Here, the authors demonstrate a bottom-up evolution route of electrochemically reducing Cs3Rh2I9 halide-perovskite clusters to prepare ultrafine Rh nanoparticles with multiply sites for alkaline hydrogen evolution.