Inverted optical bistability and optical limiting in coherently driven exciton–polaritons

Abstract

Exciton–polaritons in optical cavities exhibit strong nonlinearities predominantly because of the third-order Kerr-like interactions mediated by the excitonic component. Under quasi-resonant excitation, depending on the energy of the incident laser, it results in the optical limiting or bistable behavior. The latter phenomenon is manifested by the hysteresis loop observed in the input–output power characteristics, when a cavity is quasi-resonantly driven by a laser field. The direction of the loop is typically counterclockwise when increasing and subsequently decreasing the optical power. In this work, we demonstrate the optical bistability with an inverted hysteresis direction. It is observed in an exfoliated CdTe-based semiconductor microcavity when the frequency of the pumping laser is tuned slightly below the lower polariton mode. This unusual behavior is caused by the interplay of the suppression of strong coupling and the redshift of the lower polariton mode energy when increasing the incident power. We show that under these conditions, the polariton microcavity can be used as an optical limiter. All of the experimental observations, the shape and the direction of the hysteresis and the optical limiting behavior, are fully supported by a theoretical model.