Physical Review Research (Jul 2021)

Single quantum emitter Dicke enhancement

  • Tommaso Tufarelli,
  • Daniel Friedrich,
  • Heiko Groß,
  • Joachim Hamm,
  • Ortwin Hess,
  • Bert Hecht

DOI
https://doi.org/10.1103/PhysRevResearch.3.033103
Journal volume & issue
Vol. 3, no. 3
p. 033103

Abstract

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Coupling N identical emitters to the same field mode is a well-established method to enhance light-matter interaction. However, the resulting sqrt[N] boost of the coupling strength comes at the cost of a “linearized” (effectively semiclassical) dynamics. Here, we instead demonstrate a new approach for enhancing the coupling constant of a single quantum emitter, while retaining the nonlinear character of the light-matter interaction. We consider a single quantum emitter with N nearly degenerate transitions that are collectively coupled to the same field mode. We show that in such conditions an effective Jaynes-Cummings model emerges with a boosted coupling constant of order sqrt[N]. The validity and consequences of our general conclusions are analytically demonstrated for the instructive case N=2. We further observe that our system can closely match the spectral line shapes and photon autocorrelation functions typical of Jaynes-Cummings physics, proving that quantum optical nonlinearities are retained. Our findings match up very well with recent broadband plasmonic nanoresonator strong-coupling experiments and will, therefore, facilitate the control and detection of single-photon nonlinearities at ambient conditions.