CO anthropogenic emissions in Europe from 2011 to 2021: insights from Measurement of Pollution in the Troposphere (MOPITT) satellite data

Abstract

​​​​​​​We have used the variational inversion drivers of the recent Community Inversion Framework (CIF), coupled to a European configuration of the CHIMERE regional chemistry transport model and its adjoint to derive carbon monoxide (CO) emissions from Measurement of Pollution in the Troposphere (MOPITT) TIR-NIR (thermal-infrared near-infrared) observations, for a period of over 10 years from 2011 to 2021. The analysis of the inversion results reveals the challenges associated with the inversion of CO emissions at the regional scale over Europe. Annual budgets of national emissions have decreased by about 1 %–11 % over the decade and across Europe. These decreases are mainly due to negative corrections during autumn and winter. The posterior CO emissions follow a decreasing trend over the European Union and United Kingdom area of about −2.2 % yr−1, slightly lower than in the prior emissions. The assimilation of the MOPITT observation in the inversions indeed attenuates the decreasing trend of the CO emissions in the TNO inventory over areas benefiting from the highest number of MOPITT super-observations (particularly over Italy and over the Balkans), and particularly in autumn and winter. The small corrections of the CO emissions at national scales by the inversion can be attributed, first, to the general consistency between the TNO-GHGco-v3 inventory and the satellite data. Analysis of specific patterns such as the impact of the Covid-19 crisis reveals that it can also be seen as a lack of observation constraints to adjust the prior estimate of the emissions. The large errors associated with the observations in our inversion framework and the lack of data over large parts of Europe are sources of limitation on the observational constraint. Emission hotspots generate a relatively strong local signal, which is much better caught and exploited by the inversions than the larger-scale signals, despite the moderate spatial resolution of the MOPITT data. This is why the corrections of these hotspot emissions are stronger and more convincing than the corrections of the national- and continental-scale emissions. Accurate monitoring of the CO national anthropogenic emissions may thus require modelling and inversion systems at spatial resolutions finer than those used here as well as satellite images at high spatial resolution. The CO data of the TROPOMI instrument on board the Sentinel-5P mission should be well suited for such a perspective.