AIP Advances (Apr 2017)

Thickness-dependent magnetic and electrical transport properties of epitaxial La0.7Sr0.3CoO3 films

  • Binzhi Li,
  • Rajesh V. Chopdekar,
  • Alexander M. Kane,
  • Kyle Hoke,
  • Alpha T. N’Diaye,
  • Elke Arenholz,
  • Yayoi Takamura

DOI
https://doi.org/10.1063/1.4979921
Journal volume & issue
Vol. 7, no. 4
pp. 045003 – 045003-6

Abstract

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The thickness-dependent magnetic and electrical transport properties of nearly strain-free La0.7Sr0.3CoO3 (LSCO) films grown on (001)-oriented (LaAlO3)0.3 (Sr2AlTaO6)0.7 substrates were systematically studied. A crossover from ferromagnetic/metallic to non-magnetic/insulating behavior occurs at a critical thickness (∼8 nm) that is significantly smaller than LSCO films under larger strains in reported literature. X-ray absorption measurements revealed that the difference of functional properties at reduced film thicknesses was accompanied by changes in the valence state of Co ions at the film/substrate interface.