Nature Communications (Apr 2020)

Voltage- and time-dependent valence state transition in cobalt oxide catalysts during the oxygen evolution reaction

  • Jing Zhou,
  • Linjuan Zhang,
  • Yu-Cheng Huang,
  • Chung-Li Dong,
  • Hong-Ji Lin,
  • Chien-Te Chen,
  • L. H. Tjeng,
  • Zhiwei Hu

DOI
https://doi.org/10.1038/s41467-020-15925-2
Journal volume & issue
Vol. 11, no. 1
pp. 1 – 10

Abstract

Read online

Determining catalyst electronic structures during electrochemical reactions is crucial to understand mechanisms. Here authors perform in operando soft X-ray spectroscopy on a cobalt oxide catalyst during O2 evolution and observe voltage and time-dependent valence state transitions.