Scientific Reports (Nov 2023)

Indications of a ferromagnetic quantum critical point in $$\textrm{SmN}_{1-\delta }$$ SmN 1 - δ

  • W. F. Holmes-Hewett,
  • K. Van Koughnet,
  • J. D. Miller,
  • E. X. M. Trewick,
  • B. J. Ruck,
  • H. J. Trodahl,
  • R. G. Buckley

DOI
https://doi.org/10.1038/s41598-023-46911-5
Journal volume & issue
Vol. 13, no. 1
pp. 1 – 10

Abstract

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Abstract We investigate the previously observed superconductivity in ferromagnetic SmN in the context of the breakdown of order between two magnetic phases. Nitrogen vacancy doped SmN $$_{1-\delta }$$ 1 - δ is a semiconductor which lies in the intermediary between ferromagnetic SmN and anti-ferromagnetic Sm. Optical data reported here corroborate the prediction that electrical transport is mediated by Sm 4f defect states, and electrical transport measurements characterise the metal-insulator transition over the doping range. Our measurements show that the superconducting state in nitrogen vacancy doped $$\textrm{SmN}_{1-\delta }$$ SmN 1 - δ is the most robust near the breakdown of magnetic order, and indicate the location of a quantum critical point. Furthermore we provide additional evidence that the superconducting state is formed from majority spin electrons and thus of unconventional S = 1 type.