Nano-Micro Letters (Sep 2024)

Crystallization Modulation and Holistic Passivation Enables Efficient Two-Terminal Perovskite/CuIn(Ga)Se2 Tandem Solar Cells

  • Cong Geng,
  • Kuanxiang Zhang,
  • Changhua Wang,
  • Chung Hsien Wu,
  • Jiwen Jiang,
  • Fei Long,
  • Liyuan Han,
  • Qifeng Han,
  • Yi-Bing Cheng,
  • Yong Peng

DOI
https://doi.org/10.1007/s40820-024-01514-1
Journal volume & issue
Vol. 17, no. 1
pp. 1 – 11

Abstract

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Highlights Integrating perovskite solar cells onto irregular rough CuIn(Ga)Se2 (CIGS) surfaces remains a challenge; new strategy was explored to develop monolithic perovskite/CIGS tandem solar cell by manipulating the crystallization of perovskite. Surface reconstruction and field-effect passivation are developed synergistically to issue complex interface relationship between perovskite and C60. The champion power conversion efficiency (PCE) of 24.6% realized, providing significant commercial opportunities for all thin-film-based perovskite/CIGS tandem cells.

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