Optimization of energy storage properties in (1)NaBiTiO3-SrLaTiO3-relaxed ferroelectric ceramics

Ziyue Ma; Jianye Zhu; Jianhua Wu; Yanhua Hu; Xiaojie Lou; Ningning Sun; Ye Zhao; Yong Li; Xihong Hao

doi:10.1142/S2010135X22420036

Journal of Advanced Dielectrics (Feb 2023)

Optimization of energy storage properties in (1)NaBiTiO3-SrLaTiO3-relaxed ferroelectric ceramics

Ziyue Ma,
Jianye Zhu,
Jianhua Wu,
Yanhua Hu,
Xiaojie Lou,
Ningning Sun,
Ye Zhao,
Yong Li,
Xihong Hao

Affiliations

Ziyue Ma: Inner Mongolia Key Laboratory of Ferroelectric-Related New Energy Materials and Devices, School of Materials and Metallurgy, Inner Mongolia University of Science and Technology, Baotou, Inner Mongolia 014010, P. R. China
Jianye Zhu: Inner Mongolia Key Laboratory of Ferroelectric-Related New Energy Materials and Devices, School of Materials and Metallurgy, Inner Mongolia University of Science and Technology, Baotou, Inner Mongolia 014010, P. R. China
Jianhua Wu: Inner Mongolia Key Laboratory of Ferroelectric-Related New Energy Materials and Devices, School of Materials and Metallurgy, Inner Mongolia University of Science and Technology, Baotou, Inner Mongolia 014010, P. R. China
Yanhua Hu: Department of Chemical Engineering, Ordos Institute of Technology, Ordos, Inner Mongolia 017000, P. R. China
Xiaojie Lou: Frontier Institute of Science and Technology and State Key Laboratory for Mechanical Behavior of Materials Xi’an Jiaotong University, Xi’an, Shaanxi 710049, P. R. China
Ningning Sun: Inner Mongolia Key Laboratory of Ferroelectric-Related New Energy Materials and Devices, School of Materials and Metallurgy, Inner Mongolia University of Science and Technology, Baotou, Inner Mongolia 014010, P. R. China
Ye Zhao: Inner Mongolia Key Laboratory of Ferroelectric-Related New Energy Materials and Devices, School of Materials and Metallurgy, Inner Mongolia University of Science and Technology, Baotou, Inner Mongolia 014010, P. R. China
Yong Li: Inner Mongolia Key Laboratory of Ferroelectric-Related New Energy Materials and Devices, School of Materials and Metallurgy, Inner Mongolia University of Science and Technology, Baotou, Inner Mongolia 014010, P. R. China
Xihong Hao: Inner Mongolia Key Laboratory of Ferroelectric-Related New Energy Materials and Devices, School of Materials and Metallurgy, Inner Mongolia University of Science and Technology, Baotou, Inner Mongolia 014010, P. R. China

DOI: https://doi.org/10.1142/S2010135X22420036
Journal volume & issue: Vol. 13, no. 01

Abstract

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Ferroelectric materials are considered to be the most competitive energy storage materials for applications in pulsed power electronics due to excellent charge–discharge properties. However, the low energy storage density is the primary problem limiting their practical application. In this study, (1[Formula: see text])Na[Formula: see text]Bi[Formula: see text]TiO3–[Formula: see text]Sr[Formula: see text]La[Formula: see text]TiO3[(1[Formula: see text])NBT–[Formula: see text]SLT] ferroelectric ceramics are found to exhibit excellent energy storage performances through a synergistic strategy. As the SLT concentration increases, the relaxation characteristic increases significantly and the breakdown strength increases dramatically from 150 kV/cm to 220 kV/cm. The recoverable energy storage density of the 0.55NBT–0.45SLT ceramic is 2.86 J/cm3 with an energy storage efficiency of 88% under an electric field of 220 kV/cm. Furthermore, the ceramic with [Formula: see text] = 0.45 mol exhibited excellent energy storage stability in the ranges of 20–180[Formula: see text]C (temperature) and 1–125 Hz (frequency). These excellent properties demonstrate the potential of (1[Formula: see text])NBT–[Formula: see text]SLT ceramics when used as dielectric capacitors in pulsed power systems.

Published in Journal of Advanced Dielectrics

ISSN: 2010-135X (Print); 2010-1368 (Online)
Publisher: World Scientific Publishing
Country of publisher: Singapore
LCC subjects: Science: Physics: Electricity and magnetism: Electricity
Website: http://www.worldscientific.com/worldscinet/jad

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