Beilstein Journal of Nanotechnology (Apr 2018)

Room-temperature single-photon emitters in titanium dioxide optical defects

  • Kelvin Chung,
  • Yu H. Leung,
  • Chap H. To,
  • Aleksandra B. Djurišić,
  • Snjezana Tomljenovic-Hanic

DOI
https://doi.org/10.3762/bjnano.9.100
Journal volume & issue
Vol. 9, no. 1
pp. 1085 – 1094

Abstract

Read online

Fluorescence properties of crystallographic point defects within different morphologies of titanium dioxide were investigated. For the first time, room-temperature single-photon emission in titanium dioxide optical defects was discovered in thin films and commercial nanoparticles. Three-level defects were identified because the g(2) correlation data featured prominent shoulders around the antibunching dip. Stable and blinking photodynamics were observed for the single-photon emitters. These results reveal a new room-temperature single-photon source within a wide bandgap semiconductor.

Keywords