Enhanced optical transmittance and room temperature ferromagnetism in Al-doped zinc oxide epitaxial films

Abstract

We present a systematic investigation of the detailed structural, optical and magnetic properties of ZnO thin films deposited by pulsed laser deposition as a function of varying Al doping from 0% to 5%. The observed features can be associated with strain introduced into the ZnO lattice by the incorporation of Al. Enhanced optical transmittance values close to 95% were achieved in Al-doped ZnO epitaxial films deposited on sapphire substrates. In addition, these films exhibit robust ferromagnetic properties at room temperature with saturation magnetization that varies from 143 to 63 emu/cm3 for Al dopant concentrations from 0% to 5%. It is demonstrated that the saturation magnetization is related to the strain introduced into the lattice with increased Al doping.