Photonics (Mar 2024)

Cascaded Third-Harmonic Generation in Optically Induced 3D Nonlinear Photonic Crystals

  • Tianxiang Xu,
  • Sen Wang,
  • Jing Zeng,
  • Dawei Liu,
  • Ruwei Zhao,
  • Yuming Yao,
  • Yuhao Zhao,
  • Hui Zhao,
  • Tiefeng Xu,
  • Yan Sheng

DOI
https://doi.org/10.3390/photonics11040313
Journal volume & issue
Vol. 11, no. 4
p. 313

Abstract

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Nonlinear photonic crystals with 3D orthorhombic lattice structures were fabricated using the femtosecond laser-poling technique in ferroelectric Sr0.28Ba0.72Nb2O6 (SBN) crystals. The crystals were used to demonstrate the possibility of generating cascaded third-harmonic waves in optically poled ferroelectric structures. The spectral response and conversion efficiency of the third-harmonic process were experimentally investigated. While the nonlinear cascading processes can be commonly realized in electric-field-poled ferroelectric crystals, their generation in optically poled ferroelectric domain structures have not been reported elsewhere. In addition to the fully phase-matched nonlinear interaction, Cherenkov-type third-harmonic generation that fulfills the longitudinal phase-matching condition was also experimentally studied. Our study contributes to exploring the full potential of optically induced nonlinear photonic crystals and provides a new choice of materials for third-harmonic generation.

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