Recent advances in high-order harmonic generation from laser-ablated plumes at the advanced laser light source laboratory

Abstract

High-order harmonic generation is a nonlinear optical frequency conversion process that occurs during intense ultrafast laser-matter interaction. At the Advanced Laser Light Source laboratory, we use ultrafast laser pulses having diverse wavelengths, spanning visible, near- and mid-infrared ranges, to generate high-order harmonics from laser-ablated plumes in the extreme ultraviolet or soft X-ray region of the electromagnetic spectrum. The Advanced Laser Light Source Laboratory is situated within the Énergie Matériaux Télécommunications Center of the Institut national de la recherche scientifique in Montréal, Quebec, Canada. We focus on generating bright and broadband harmonics by exploiting various types of ultrafast resonances in different species within the laser-ablated plume, and use them for applications in ultrafast spectroscopy, imaging, and AMO science. We are also actively exploring previously unknown physics governing the harmonic generation from different resonances. In this review article, we provide an overview of the recent advancements made in these directions.

Keywords

• High-order harmonic generation
• Laser-ablated plume
• Resonant harmonic
• Intense XUV source