Enhancing the Electrocatalytic Oxidation of 5-Hydroxymethylfurfural Through Cascade Structure Tuning for Highly Stable Biomass Upgrading

Xiaoli Jiang; Xianhui Ma; Yuanteng Yang; Yang Liu; Yanxia Liu; Lin Zhao; Penglei Wang; Yagang Zhang; Yue Lin; Yen Wei

doi:10.1007/s40820-024-01493-3

Nano-Micro Letters (Aug 2024)

Enhancing the Electrocatalytic Oxidation of 5-Hydroxymethylfurfural Through Cascade Structure Tuning for Highly Stable Biomass Upgrading

Xiaoli Jiang,
Xianhui Ma,
Yuanteng Yang,
Yang Liu,
Yanxia Liu,
Lin Zhao,
Penglei Wang,
Yagang Zhang,
Yue Lin,
Yen Wei

Affiliations

Xiaoli Jiang: School of Materials and Energy, University of Electronic Science and Technology of China
Xianhui Ma: Hefei National Research Center for Physical Sciences at the Microscale, University of Science and Technology of China
Yuanteng Yang: School of Materials and Energy, University of Electronic Science and Technology of China
Yang Liu: School of Materials and Energy, University of Electronic Science and Technology of China
Yanxia Liu: School of Materials and Energy, University of Electronic Science and Technology of China
Lin Zhao: School of Materials and Energy, University of Electronic Science and Technology of China
Penglei Wang: School of Materials and Energy, University of Electronic Science and Technology of China
Yagang Zhang: School of Materials and Energy, University of Electronic Science and Technology of China
Yue Lin: Hefei National Research Center for Physical Sciences at the Microscale, University of Science and Technology of China
Yen Wei: The Key Laboratory of Bioorganic Phosphorus Chemistry and Chemical Biology (Ministry of Education), Department of Chemistry, Tsinghua University

DOI: https://doi.org/10.1007/s40820-024-01493-3
Journal volume & issue: Vol. 16, no. 1
pp. 1 – 19

Abstract

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Highlights A novel cascade strategy is proposed to construct Pd-NiCo2O4 electrocatalyst. First time discovery that Ni incorporation together with Pd loading is able to balance the competitive adsorption of OH– and 5-hydroxymethylfurfural. Pd–NiCo2O4 promotes both the indirect and direct synergistic oxidation process. Pd–NiCo2O4 catalyst exhibits extraordinary current density and excellent Faradaic Efficiency at a low potential.

Published in Nano-Micro Letters

ISSN: 2311-6706 (Print); 2150-5551 (Online)
Publisher: SpringerOpen
Country of publisher: Germany
LCC subjects: Technology
Website: http://www.springer.com/40820

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