Magnetic field induced competing phases in spin-orbital entangled Kitaev magnets

Abstract

There has been a great interest in magnetic field induced quantum spin liquids in Kitaev magnets after the discovery of neutron scattering continuum and half-quantized thermal Hall conductivity in the material α-RuCl_{3}. In this work, we provide a semiclassical analysis of the relevant theoretical models, which enable us to treat large system sizes approximating the thermodynamic limit. We find a series of competing magnetic orders with fairly large unit cells at intermediate magnetic fields, which are mostly missed by previous studies. We show that quantum fluctuations are typically strong in these large unit cell orders, while the magnetic excitations, magnons, have a dispersion that resembles a scattering continuum. The huge quantity of magnon bands with finite Chern numbers also gives rise to an unusually large thermal Hall conductivity. Given the highly frustrated nature of the spin model, the large unit cell orders are likely to melt into the putative spin liquid in the quantum limit. Our work provides an important basis for a thorough investigation of emergent spin liquids and competing phases in Kitaev magnets.