Atmospheric Chemistry and Physics (Mar 2008)
Modelling sea salt aerosol and its direct and indirect effects on climate
Abstract
A size-dependent sea salt aerosol parameterization was developed based on the piecewise log-normal approximation (PLA) for aerosol size distributions. Results of this parameterization from simulations with a global climate model produce good agreement with observations at the surface and for vertically-integrated volume size distributions. The global and annual mean of the sea salt burden is 10.1 mg m<sup>−2</sup>. The direct radiative forcing is calculated to be −1.52 and −0.60 W m<sup>−2</sup> for clear sky and all sky, respectively. The first indirect radiative forcing is about twice as large as the direct forcing for all-sky (−1.34 W m<sup>−2</sup>). The results also show that the total indirect forcing of sea salt is −2.9 W m<sup>−2</sup> if climatic feedbacks are taken into account. The sensitivity of the forcings to changes in the burdens and sizes of sea salt particles was also investigated based on additional simulations with a different sea salt source function.