Spin pinning effect to reconstructed oxyhydroxide layer on ferromagnetic oxides for enhanced water oxidation

Abstract

Water oxidation to triplet oxygen requires a spin polarization process for faster kinetics. Here, the authors show an interface spin pinning effect between ferromagnetic oxides and reconstructed oxyhydroxide surface layer, where the spin ordering in paramagnetic oxyhydroxide catalyst layer can be tuned to improve the intrinsic activity.