Accelerated water activation and stabilized metal-organic framework via constructing triangular active-regions for ampere-level current density hydrogen production

Fanpeng Cheng; Xianyun Peng; Lingzi Hu; Bin Yang; Zhongjian Li; Chung-Li Dong; Jeng-Lung Chen; Liang-Ching Hsu; Lecheng Lei; Qiang Zheng; Ming Qiu; Liming Dai; Yang Hou

doi:10.1038/s41467-022-34278-6

Nature Communications (Oct 2022)

Accelerated water activation and stabilized metal-organic framework via constructing triangular active-regions for ampere-level current density hydrogen production

Fanpeng Cheng,
Xianyun Peng,
Lingzi Hu,
Bin Yang,
Zhongjian Li,
Chung-Li Dong,
Jeng-Lung Chen,
Liang-Ching Hsu,
Lecheng Lei,
Qiang Zheng,
Ming Qiu,
Liming Dai,
Yang Hou

Affiliations

Fanpeng Cheng: Key Laboratory of Biomass Chemical Engineering of Ministry of Education, College of Chemical and Biological Engineering, Zhejiang University
Xianyun Peng: Institute of Zhejiang University - Quzhou
Lingzi Hu: Institute of Nanoscience and Nanotechnology, College of Physical Science and Technology, Central China Normal University
Bin Yang: Key Laboratory of Biomass Chemical Engineering of Ministry of Education, College of Chemical and Biological Engineering, Zhejiang University
Zhongjian Li: Key Laboratory of Biomass Chemical Engineering of Ministry of Education, College of Chemical and Biological Engineering, Zhejiang University
Chung-Li Dong: Department of Physics, Tamkang University
Jeng-Lung Chen: National Synchrotron Radiation Research Center
Liang-Ching Hsu: National Synchrotron Radiation Research Center
Lecheng Lei: Key Laboratory of Biomass Chemical Engineering of Ministry of Education, College of Chemical and Biological Engineering, Zhejiang University
Qiang Zheng: CAS Key Laboratory of Standardization and Measurement for Nanotechnology, CAS Center for Excellence in Nanoscience, National Center for Nanoscience and Technology
Ming Qiu: Institute of Nanoscience and Nanotechnology, College of Physical Science and Technology, Central China Normal University
Liming Dai: Australian Carbon Materials Centre (A-CMC), School of Chemical Engineering, University of New South Wales
Yang Hou: Key Laboratory of Biomass Chemical Engineering of Ministry of Education, College of Chemical and Biological Engineering, Zhejiang University

DOI: https://doi.org/10.1038/s41467-022-34278-6
Journal volume & issue: Vol. 13, no. 1
pp. 1 – 10

Abstract

Read online

The sluggish water activation kinetics and instability of metal-organic frameworks for hydrogen evolution reaction limit their industrial applications. Here, authors construct a unique triangular active region to accelerate the crucial water activation and stabilize metal-organic frameworks.

Published in Nature Communications

ISSN: 2041-1723 (Online)
Publisher: Nature Portfolio
Country of publisher: United Kingdom
LCC subjects: Science
Website: https://www.nature.com/ncomms/

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