Energy cascades in donor-acceptor exciton-polaritons observed by ultrafast two-dimensional white-light spectroscopy

Minjung Son; Zachary T. Armstrong; Ryan T. Allen; Abitha Dhavamani; Michael S. Arnold; Martin T. Zanni

doi:10.1038/s41467-022-35046-2

Nature Communications (Nov 2022)

Energy cascades in donor-acceptor exciton-polaritons observed by ultrafast two-dimensional white-light spectroscopy

Minjung Son,
Zachary T. Armstrong,
Ryan T. Allen,
Abitha Dhavamani,
Michael S. Arnold,
Martin T. Zanni

Affiliations

Minjung Son: Department of Chemistry, University of Wisconsin-Madison
Zachary T. Armstrong: Department of Chemistry, University of Wisconsin-Madison
Ryan T. Allen: Department of Chemistry, University of Wisconsin-Madison
Abitha Dhavamani: Department of Materials Science and Engineering, University of Wisconsin-Madison
Michael S. Arnold: Department of Materials Science and Engineering, University of Wisconsin-Madison
Martin T. Zanni: Department of Chemistry, University of Wisconsin-Madison

DOI: https://doi.org/10.1038/s41467-022-35046-2
Journal volume & issue: Vol. 13, no. 1
pp. 1 – 10

Abstract

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Exciton-polaritons are hybridized light-matter states that exhibit intriguing phenomena that are unobserved in purely excitonic states. Here, the authors elucidate the photophysical mechanism of polariton-assisted long-range energy transfer in carbon nanotubes using two-dimensional white-light spectroscopy and quantum calculations.

Published in Nature Communications

ISSN: 2041-1723 (Online)
Publisher: Nature Portfolio
Country of publisher: United Kingdom
LCC subjects: Science
Website: https://www.nature.com/ncomms/

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