AIP Advances (Apr 2019)

Plasmon-exciton coupling in nanostructured metal-semiconductor composite films

  • Viktoriia V. Savchuk,
  • Roman V. Gamernyk,
  • Ihor S. Virt,
  • Serhiy Z. Malynych,
  • Anatoliy O. Pinchuk

DOI
https://doi.org/10.1063/1.5090900
Journal volume & issue
Vol. 9, no. 4
pp. 045021 – 045021-6

Abstract

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Nonlinear optical response of metal-semiconductor Zn0.8Co0.2O/Au nanocomposite films was studied experimentally and theoretically. Z-scan measurements revealed a positive nonlinear index of refraction of the composite film. Fluorescent spectroscopy measurements exhibited a narrow sharp peak that might be attributed to exciton peak of semiconductor nanostructured thin film enhanced by nearby gold nanoparticles. Classical electrodynamic calculations of a quantum dot in close proximity to a gold nanoparticle agree well with the experimentally observed normalized quantum efficiency.