Direction control of colloidal quantum dot emission using dielectric metasurfaces

Abstract

Owing to the recent developments of dielectric metasurfaces, their applications have been expanding from those pertaining to the thickness shrinkage of passive optical elements, such as lenses, polarizers, and quarter-wave plates, to applications pertaining to their integration with active optical devices, such as vertical-cavity surface-emitting lasers. Even though directional lasing and beam shaping of laser emission have been successfully demonstrated, the integration of metasurfaces with random light sources, such as light-emitting diodes, is limited because of function and efficiency issues attributed to the fact that metasurfaces are basically based on the resonance property of the nanostructure. To control the direction of emission from colloidal quantum dots, we present a dielectric metasurface deflector composed of two asymmetric TiO2 nanoposts. TiO2 deflector arrays were fabricated with a dry etching method that is adaptive to mass production and integrated with a colloidal quantum dot resonant cavity formed by sandwiching two distributed Bragg reflectors. To ensure the deflection ability of the fabricated sample, we measured the photoluminescence and far-field patterns of emission from the resonant cavity. From the obtained results, we demonstrated that the colloidal quantum dot emission transmitted through our deflector arrays was deflected by 18°, and the efficiency of deflection was 71% with respect to the emission from the resonant cavity. This integration of dielectric metasurfaces with a resonant cavity shows the possibility of expanding the application of visible metasurfaces in active devices and may help to develop next-generation active devices with novel functions.

Keywords

• asymmetric nanopost array
• colloidal quantum dot
• dielectric metasurface
• light-emitting diode
• resonant cavity
• tio2 dry etching