Scientific Reports (Aug 2023)

Thermal properties and mechanical behavior of hot pressed PEEK/graphite thin film laminate composites

  • Bakytzhan Sariyev,
  • Alina Abdikadyr,
  • Temirlan Baitikenov,
  • Yerbolat Anuarbekov,
  • Boris Golman,
  • Christos Spitas

DOI
https://doi.org/10.1038/s41598-023-39905-w
Journal volume & issue
Vol. 13, no. 1
pp. 1 – 12

Abstract

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Abstract This work studies high-performance laminate composite materials made of graphite and poly(ether-ether-ketone) (PEEK). The main objective was to enhance graphite's inherent properties by the addition of PEEK to produce materials with improved thermal and mechanical stability for high-performance applications. The composites were fabricated using a hot press method at a temperature below 310 °C. The newly formed materials were then subjected to various tests, including Scanning Electron Microscopy, Thermogravimetric Analysis, mechanical properties tests, nanoindentation tests, and X-Ray Diffraction to assess their structural, thermal, and mechanical properties. Our findings showed a substantial interfacial interaction between PEEK and graphite, indicating successful composite formation. Both three-layered PEEK/graphite/PEEK (PGP) and five-layered PEEK/graphite/PEEK/graphite/PEEK (PG)2P composites exhibited superior thermal stability at high temperatures compared to neat PEEK. Moreover, our mechanical tests demonstrated a 172% increase in ultimate tensile strength of PGP compared to neat graphite. Additionally, nanoindentation tests confirmed an increase in both Young's modulus and hardness of composites. Furthermore, XRD analysis revealed a 35.5% increase in crystallinity in the fabricated composites compared to pristine PEEK. These findings significantly contribute to the field of high-performance composite materials, confirming that the hot pressing of PEEK and graphite sheets results in enhanced thermal and mechanical properties.