Nature Communications (Mar 2023)

Real-time insight into the multistage mechanism of nanoparticle exsolution from a perovskite host surface

  • Eleonora Calì,
  • Melonie P. Thomas,
  • Rama Vasudevan,
  • Ji Wu,
  • Oriol Gavalda-Diaz,
  • Katharina Marquardt,
  • Eduardo Saiz,
  • Dragos Neagu,
  • Raymond R. Unocic,
  • Stephen C. Parker,
  • Beth S. Guiton,
  • David J. Payne

DOI
https://doi.org/10.1038/s41467-023-37212-6
Journal volume & issue
Vol. 14, no. 1
pp. 1 – 10

Abstract

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The separation of nanoparticles from oxide hosts by exsolution forms the basis for catalytic and energy-related applications. Here, the authors elucidate the multistep mechanism of exsolution at perovskite surfaces by combining real-time electron microscopy and computational methods.