Nature Communications (May 2019)
Real-time observation of X-ray-induced intramolecular and interatomic electronic decay in CH2I2
- Hironobu Fukuzawa,
- Tsukasa Takanashi,
- Edwin Kukk,
- Koji Motomura,
- Shin-ichi Wada,
- Kiyonobu Nagaya,
- Yuta Ito,
- Toshiyuki Nishiyama,
- Christophe Nicolas,
- Yoshiaki Kumagai,
- Denys Iablonskyi,
- Subhendu Mondal,
- Tetsuya Tachibana,
- Daehyun You,
- Syuhei Yamada,
- Yuta Sakakibara,
- Kazuki Asa,
- Yuhiro Sato,
- Tsukasa Sakai,
- Kenji Matsunami,
- Takayuki Umemoto,
- Kango Kariyazono,
- Shinji Kajimoto,
- Hikaru Sotome,
- Per Johnsson,
- Markus S. Schöffler,
- Gregor Kastirke,
- Kuno Kooser,
- Xiao-Jing Liu,
- Theodor Asavei,
- Liviu Neagu,
- Serguei Molodtsov,
- Kohei Ochiai,
- Manabu Kanno,
- Kaoru Yamazaki,
- Shigeki Owada,
- Kanade Ogawa,
- Tetsuo Katayama,
- Tadashi Togashi,
- Kensuke Tono,
- Makina Yabashi,
- Aryya Ghosh,
- Kirill Gokhberg,
- Lorenz S. Cederbaum,
- Alexander I. Kuleff,
- Hiroshi Fukumura,
- Naoki Kishimoto,
- Artem Rudenko,
- Catalin Miron,
- Hirohiko Kono,
- Kiyoshi Ueda
Affiliations
- Hironobu Fukuzawa
- Institute of Multidisciplinary Research for Advanced Materials, Tohoku University
- Tsukasa Takanashi
- Institute of Multidisciplinary Research for Advanced Materials, Tohoku University
- Edwin Kukk
- Department of Physics and Astronomy, University of Turku
- Koji Motomura
- Institute of Multidisciplinary Research for Advanced Materials, Tohoku University
- Shin-ichi Wada
- RIKEN SPring-8 Center
- Kiyonobu Nagaya
- RIKEN SPring-8 Center
- Yuta Ito
- Institute of Multidisciplinary Research for Advanced Materials, Tohoku University
- Toshiyuki Nishiyama
- Department of Physics, Kyoto University
- Christophe Nicolas
- Synchrotron SOLEIL, L’Orme des Merisiers, Saint-Aubin, BP 48
- Yoshiaki Kumagai
- Institute of Multidisciplinary Research for Advanced Materials, Tohoku University
- Denys Iablonskyi
- Institute of Multidisciplinary Research for Advanced Materials, Tohoku University
- Subhendu Mondal
- Institute of Multidisciplinary Research for Advanced Materials, Tohoku University
- Tetsuya Tachibana
- Institute of Multidisciplinary Research for Advanced Materials, Tohoku University
- Daehyun You
- Institute of Multidisciplinary Research for Advanced Materials, Tohoku University
- Syuhei Yamada
- Institute of Multidisciplinary Research for Advanced Materials, Tohoku University
- Yuta Sakakibara
- Institute of Multidisciplinary Research for Advanced Materials, Tohoku University
- Kazuki Asa
- Department of Physics, Kyoto University
- Yuhiro Sato
- Department of Physics, Kyoto University
- Tsukasa Sakai
- Department of Physics, Kyoto University
- Kenji Matsunami
- Department of Physics, Kyoto University
- Takayuki Umemoto
- Department of Physical Science, Hiroshima University
- Kango Kariyazono
- Department of Physical Science, Hiroshima University
- Shinji Kajimoto
- Department of Chemistry, Graduate School of Science, Tohoku University
- Hikaru Sotome
- Department of Chemistry, Graduate School of Science, Tohoku University
- Per Johnsson
- Department of Physics, Lund University
- Markus S. Schöffler
- Institut für Kernphysik, J.W. Goethe Universität
- Gregor Kastirke
- Institut für Kernphysik, J.W. Goethe Universität
- Kuno Kooser
- Department of Physics and Astronomy, University of Turku
- Xiao-Jing Liu
- School of Physics and Nuclear Energy Engineering, Beihang University
- Theodor Asavei
- Extreme Light Infrastructure - Nuclear Physics (ELI-NP), “Horia Hulubei” National Institute for Physics and Nuclear Engineering
- Liviu Neagu
- Extreme Light Infrastructure - Nuclear Physics (ELI-NP), “Horia Hulubei” National Institute for Physics and Nuclear Engineering
- Serguei Molodtsov
- European XFEL GmbH, Holzkoppel 4
- Kohei Ochiai
- Department of Chemistry, Graduate School of Science, Tohoku University
- Manabu Kanno
- Department of Chemistry, Graduate School of Science, Tohoku University
- Kaoru Yamazaki
- Institute for Materials Research, Tohoku University
- Shigeki Owada
- RIKEN SPring-8 Center
- Kanade Ogawa
- RIKEN SPring-8 Center
- Tetsuo Katayama
- Japan Synchrotron Radiation Research Institute (JASRI), Sayo
- Tadashi Togashi
- Japan Synchrotron Radiation Research Institute (JASRI), Sayo
- Kensuke Tono
- Japan Synchrotron Radiation Research Institute (JASRI), Sayo
- Makina Yabashi
- RIKEN SPring-8 Center
- Aryya Ghosh
- Theoretical Chemistry, PCI, Universität Heidelberg
- Kirill Gokhberg
- Theoretical Chemistry, PCI, Universität Heidelberg
- Lorenz S. Cederbaum
- Theoretical Chemistry, PCI, Universität Heidelberg
- Alexander I. Kuleff
- Theoretical Chemistry, PCI, Universität Heidelberg
- Hiroshi Fukumura
- Department of Chemistry, Graduate School of Science, Tohoku University
- Naoki Kishimoto
- Department of Chemistry, Graduate School of Science, Tohoku University
- Artem Rudenko
- J. R. Macdonald Laboratory, Department of Physics, Kansas State University
- Catalin Miron
- Synchrotron SOLEIL, L’Orme des Merisiers, Saint-Aubin, BP 48
- Hirohiko Kono
- Department of Chemistry, Graduate School of Science, Tohoku University
- Kiyoshi Ueda
- Institute of Multidisciplinary Research for Advanced Materials, Tohoku University
- DOI
- https://doi.org/10.1038/s41467-019-10060-z
- Journal volume & issue
-
Vol. 10,
no. 1
pp. 1 – 8
Abstract
Understanding strong X-ray induced phenomena is important for applications of X-ray free-electron laser imaging. Here, the authors show time-resolved measurements of X-ray free-electron laser induced electronic decay of CH2I2 molecule probed with NIR pulses and identify mechanisms behind different transient states lifetimes.
