Joule self-heating effects and controlling oxygen vacancy in La0.8Ba0.2MnO3 ultrathin films with nano-sized labyrinth morphology

Abstract

Electric current induced Joule heating effects have been investigated in La0.8Ba0.2MnO3 ultrathin films deposited on a LaAlO3(001) single crystal substrate with a smaller lattice constant by using the sol–gel method. By applying moderate bias currents (∼10 mA), it is found that Joule self-heating simply gives rise to a temperature deviation between the thermostat and the test sample, but the intrinsic ρ(T) relationship measured at a low current (0.1 mA) changes a little. However, it is noteworthy that the low-temperature transport behavior degrades from the metallic to the insulating state after applying higher bias currents (>31 mA) in vacuum. Furthermore, the metallic transport can be recovered by placing the degraded film in air. The results clearly suggest that the oxygen vacancy in the La0.8Ba0.2MnO3 films is controllable in different atmospheres, particularly with the aid of the Joule self-heating. According to the SEM images, we attribute the controlled oxygen vacancy to the nano-sized labyrinth pattern of the films, where the large surface-to-volume ratio plays a crucial role.