Distinctive aerosol–cloud–precipitation interactions in marine boundary layer clouds from the ACE-ENA and SOCRATES aircraft field campaigns

Abstract

The aerosol–cloud–precipitation interactions within the cloud-topped marine boundary layer (MBL) are examined using aircraft in situ measurements from Aerosol and Cloud Experiments in the Eastern North Atlantic (ACE-ENA) and Southern Ocean Clouds, Radiation, Aerosol Transport Experimental Study (SOCRATES) field campaigns. SOCRATES clouds exhibit a larger number concentration and smaller cloud droplet effective radius (148.3 cm−3 and 8.0 µm) compared to ACE-ENA summertime (89.4 cm−3 and 9.0 µm) and wintertime clouds (70.6 cm−3 and 9.8 µm). The ACE-ENA clouds, especially during the winter, feature stronger drizzle formation via droplet growth through enhanced collision–coalescence that is attributed to a relatively cleaner environment and deeper cloud layer. Furthermore, the aerosol–cloud interaction (ACI) indices from the two aircraft field campaigns exhibit distinct sensitivities, indicating different cloud microphysical responses to aerosols. The ACE-ENA winter season features relatively fewer aerosols, which are more likely activated into cloud droplets under the conditions of sufficient water vapor availability and strong turbulence. The enriched aerosol loading during ACE-ENA summer and SOCRATES generally leads to smaller cloud droplets competing for the limited water vapor and exhibiting a stronger ACI. Notably, the precipitation susceptibilities are stronger during the ACE-ENA than during the SOCRATES campaigns. The in-cloud drizzle behavior significantly alters sub-cloud cloud condensation nuclei (CCN) budgets through the coalescence-scavenging effect and, in turn, impacts the ACI assessments. The results of this study can enhance understanding and aid in future model simulation and assessment of the aerosol–cloud interaction.