Rotational and nuclear-spin level dependent photodissociation dynamics of H2S

Yarui Zhao; Zijie Luo; Yao Chang; Yucheng Wu; Su-e Zhang; Zhenxing Li; Hongbin Ding; Guorong Wu; Jyoti S. Campbell; Christopher S. Hansen; Stuart W. Crane; Colin M. Western; Michael N. R. Ashfold; Kaijun Yuan; Xueming Yang

doi:10.1038/s41467-021-24782-6

Nature Communications (Jul 2021)

Rotational and nuclear-spin level dependent photodissociation dynamics of H2S

Yarui Zhao,
Zijie Luo,
Yao Chang,
Yucheng Wu,
Su-e Zhang,
Zhenxing Li,
Hongbin Ding,
Guorong Wu,
Jyoti S. Campbell,
Christopher S. Hansen,
Stuart W. Crane,
Colin M. Western,
Michael N. R. Ashfold,
Kaijun Yuan,
Xueming Yang

Affiliations

Yarui Zhao: School of Physics, Key Laboratory of Materials Modification by Laser, Ion and Electron Beams, Chinese Ministry of Education, Dalian University of Technology
Zijie Luo: State Key Laboratory of Molecular Reaction Dynamics and Dalian Coherent Light Source, Dalian Institute of Chemical Physics, Chinese Academy of Sciences
Yao Chang: State Key Laboratory of Molecular Reaction Dynamics and Dalian Coherent Light Source, Dalian Institute of Chemical Physics, Chinese Academy of Sciences
Yucheng Wu: State Key Laboratory of Molecular Reaction Dynamics and Dalian Coherent Light Source, Dalian Institute of Chemical Physics, Chinese Academy of Sciences
Su-e Zhang: State Key Laboratory of Molecular Reaction Dynamics and Dalian Coherent Light Source, Dalian Institute of Chemical Physics, Chinese Academy of Sciences
Zhenxing Li: State Key Laboratory of Molecular Reaction Dynamics and Dalian Coherent Light Source, Dalian Institute of Chemical Physics, Chinese Academy of Sciences
Hongbin Ding: School of Physics, Key Laboratory of Materials Modification by Laser, Ion and Electron Beams, Chinese Ministry of Education, Dalian University of Technology
Guorong Wu: State Key Laboratory of Molecular Reaction Dynamics and Dalian Coherent Light Source, Dalian Institute of Chemical Physics, Chinese Academy of Sciences
Jyoti S. Campbell: School of Chemistry, University of New South Wales
Christopher S. Hansen: School of Chemistry, University of New South Wales
Stuart W. Crane: School of Chemistry, University of Bristol
Colin M. Western: School of Chemistry, University of Bristol
Michael N. R. Ashfold: School of Chemistry, University of Bristol
Kaijun Yuan: State Key Laboratory of Molecular Reaction Dynamics and Dalian Coherent Light Source, Dalian Institute of Chemical Physics, Chinese Academy of Sciences
Xueming Yang: State Key Laboratory of Molecular Reaction Dynamics and Dalian Coherent Light Source, Dalian Institute of Chemical Physics, Chinese Academy of Sciences

DOI: https://doi.org/10.1038/s41467-021-24782-6
Journal volume & issue: Vol. 12, no. 1
pp. 1 – 10

Abstract

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The photodissociation dynamics of small molecules in the vacuum ultraviolet range can have key implications for astrochemical modelling, but revealing such dynamical details is a challenging task. Here the authors, combining high resolution experimental techniques, provide a detailed description of the fragmentation dynamics of selected rotational levels of a predissociated Rydberg state of H2S.

Published in Nature Communications

ISSN: 2041-1723 (Online)
Publisher: Nature Portfolio
Country of publisher: United Kingdom
LCC subjects: Science
Website: https://www.nature.com/ncomms/

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