Nature Communications (May 2022)

Water coordinated on Cu(I)-based catalysts is the oxygen source in CO2 reduction to CO

  • Yajun Zheng,
  • Hedan Yao,
  • Ruinan Di,
  • Zhicheng Xiang,
  • Qiang Wang,
  • Fangfang Lu,
  • Yu Li,
  • Guangxing Yang,
  • Qiang Ma,
  • Zhiping Zhang

DOI
https://doi.org/10.1038/s41467-022-30289-5
Journal volume & issue
Vol. 13, no. 1
pp. 1 – 11

Abstract

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Understanding the underlying mechanisms for catalytic reduction of CO2 over Cu based catalysts remains challenging. Here, the authors develop an effective method to reveal the vital roles of H2O in promoting metal catalysts to CO2 reduction via a modified triple stage quadrupole mass spectrometer.