Nature Communications (Sep 2020)

Atomically-precise dopant-controlled single cluster catalysis for electrochemical nitrogen reduction

  • Chuanhao Yao,
  • Na Guo,
  • Shibo Xi,
  • Cong-Qiao Xu,
  • Wei Liu,
  • Xiaoxu Zhao,
  • Jing Li,
  • Hanyan Fang,
  • Jie Su,
  • Zhongxin Chen,
  • Huan Yan,
  • Zhizhan Qiu,
  • Pin Lyu,
  • Cheng Chen,
  • Haomin Xu,
  • Xinnan Peng,
  • Xinzhe Li,
  • Bin Liu,
  • Chenliang Su,
  • Stephen J. Pennycook,
  • Cheng-Jun Sun,
  • Jun Li,
  • Chun Zhang,
  • Yonghua Du,
  • Jiong Lu

DOI
https://doi.org/10.1038/s41467-020-18080-w
Journal volume & issue
Vol. 11, no. 1
pp. 1 – 10

Abstract

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The fabrication of singly dispersed metal cluster catalysts with atomic-level control of dopants is a long-standing challenge. Here, the authors report a strategy for the synthesis of a precisely doped single cluster catalyst which shows exceptional activity for electrochemical dinitrogen reduction.