Nanoscale heterogeneity of ultrafast many-body carrier dynamics in triple cation perovskites

Jun Nishida; Peter T. S. Chang; Jiselle Y. Ye; Prachi Sharma; Dylan M. Wharton; Samuel C. Johnson; Sean E. Shaheen; Markus B. Raschke

doi:10.1038/s41467-022-33935-0

Nature Communications (Nov 2022)

Nanoscale heterogeneity of ultrafast many-body carrier dynamics in triple cation perovskites

Jun Nishida,
Peter T. S. Chang,
Jiselle Y. Ye,
Prachi Sharma,
Dylan M. Wharton,
Samuel C. Johnson,
Sean E. Shaheen,
Markus B. Raschke

Affiliations

Jun Nishida: Department of Physics, University of Colorado
Peter T. S. Chang: Department of Physics, University of Colorado
Jiselle Y. Ye: Department of Electrical, Computer, and Energy Engineering, University of Colorado
Prachi Sharma: Department of Electrical, Computer, and Energy Engineering, University of Colorado
Dylan M. Wharton: Department of Physics, University of Colorado
Samuel C. Johnson: Department of Physics, University of Colorado
Sean E. Shaheen: Department of Physics, University of Colorado
Markus B. Raschke: Department of Physics, University of Colorado

DOI: https://doi.org/10.1038/s41467-022-33935-0
Journal volume & issue: Vol. 13, no. 1
pp. 1 – 9

Abstract

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The optoelectronic performance of lead halide perovskite in highfluence applications are hindered by heterogeneous multi-polaron interactions in the nanoscale. Here, Nishda et al. spatially resolve sub-ns relaxation dynamics on the nanometer scale by ultrafast infrared pumpprobe nanoimaging.

Published in Nature Communications

ISSN: 2041-1723 (Online)
Publisher: Nature Portfolio
Country of publisher: United Kingdom
LCC subjects: Science
Website: https://www.nature.com/ncomms/

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