Electrochemical Carbon Dioxide Reduction to Ethylene: From Mechanistic Understanding to Catalyst Surface Engineering

Junpeng Qu; Xianjun Cao; Li Gao; Jiayi Li; Lu Li; Yuhan Xie; Yufei Zhao; Jinqiang Zhang; Minghong Wu; Hao Liu

doi:10.1007/s40820-023-01146-x

Nano-Micro Letters (Jul 2023)

Electrochemical Carbon Dioxide Reduction to Ethylene: From Mechanistic Understanding to Catalyst Surface Engineering

Junpeng Qu,
Xianjun Cao,
Li Gao,
Jiayi Li,
Lu Li,
Yuhan Xie,
Yufei Zhao,
Jinqiang Zhang,
Minghong Wu,
Hao Liu

Affiliations

Junpeng Qu: Joint International Laboratory on Environmental and Energy Frontier Materials, School of Environmental and Chemical Engineering, Shanghai University
Xianjun Cao: Joint International Laboratory on Environmental and Energy Frontier Materials, School of Environmental and Chemical Engineering, Shanghai University
Li Gao: Joint International Laboratory on Environmental and Energy Frontier Materials, School of Environmental and Chemical Engineering, Shanghai University
Jiayi Li: Joint International Laboratory on Environmental and Energy Frontier Materials, School of Environmental and Chemical Engineering, Shanghai University
Lu Li: Joint International Laboratory on Environmental and Energy Frontier Materials, School of Environmental and Chemical Engineering, Shanghai University
Yuhan Xie: Centre for Clean Energy Technology, Faculty of Science, University of Technology Sydney
Yufei Zhao: Joint International Laboratory on Environmental and Energy Frontier Materials, School of Environmental and Chemical Engineering, Shanghai University
Jinqiang Zhang: Centre for Clean Energy Technology, Faculty of Science, University of Technology Sydney
Minghong Wu: Joint International Laboratory on Environmental and Energy Frontier Materials, School of Environmental and Chemical Engineering, Shanghai University
Hao Liu: Centre for Clean Energy Technology, Faculty of Science, University of Technology Sydney

DOI: https://doi.org/10.1007/s40820-023-01146-x
Journal volume & issue: Vol. 15, no. 1
pp. 1 – 34

Abstract

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Highlights Three key processes in carbon dioxide reduction reaction (CO2RR) for ethylene generation were discussed, including CO2 adsorption/activation, *CO intermediates formation, and C-C coupling. The preferable mechanism for ethylene over C1 and other C2 products reaction pathways. Engineering strategies of Cu-based catalysts for CO2RR-ethylene.

Published in Nano-Micro Letters

ISSN: 2311-6706 (Print); 2150-5551 (Online)
Publisher: SpringerOpen
Country of publisher: Germany
LCC subjects: Technology
Website: http://www.springer.com/40820

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