Atmosphere (May 2023)
Effects of Aerosol Number Concentration and Updraft Velocity on Relative Dispersion during the Collision–Coalescence Growth Stage of Warm Clouds
Abstract
Relative dispersion (ɛ) is a key expression used to parameterize various cloud processes in global circulation models (GCMs) and meteorological mesoscale models. Aerosols, updraft velocity (w), and different growth stages of warm clouds are known to affect relative dispersion. A two-dimensional detailed bin microphysical cloud model is used to investigate the combined impacts of aerosol number concentration (Na) and updraft velocity on relative dispersion in the collision–coalescence stage. In addition, the causes potentially controlling the changes in ɛ with updraft velocity are explored. There are three main influence regimes: the updraft velocity main influence regime, the aerosol main influence regime, and the joint influence regime. The cause of the variations in ɛ with updraft velocity is found to be different in the three main influence regimes. In the updraft velocity main influence regime, vigorous collision–coalescence due to stronger w results in a shift in the cloud droplet number concentration spectrum toward larger droplets, and the average cloud droplet radius increases, but the spectral width is less variable, so ε decreases. In the joint influence regime, stronger cloud droplet evaporation due to the stronger dragging effect of large cloud droplets widens the spectrum, mainly by reducing the cloud droplet number concentration (Nc) of 4–30 μm, and ε increases with the reduction in w. In the aerosol main influence regime, the strongest dragging effect reduces Nc at all radii with decreasing w, and the cloud droplet number concentration spectrum (CDNCS) narrows, which becomes the formation mechanism of the positive correlation between ε and w. Evaporation mainly causes a negative correlation between ε and Nc, but weak evaporation causes the correlation to become positive under the background of high aerosol concentration. At low aerosol concentrations, a strong collision–coalescence effect leads to a negative correlation between Nc and ε, but at high aerosol concentrations, the correlation is the opposite due to a weak collision–coalescence effect.
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