Physical Review Research (Oct 2019)

Angular streaking in strong field ionization of chiral molecules

  • K. Fehre,
  • S. Eckart,
  • M. Kunitski,
  • C. Janke,
  • D. Trabert,
  • J. Rist,
  • M. Weller,
  • A. Hartung,
  • M. Pitzer,
  • L. Ph. H. Schmidt,
  • T. Jahnke,
  • R. Dörner,
  • M. S. Schöffler

DOI
https://doi.org/10.1103/PhysRevResearch.1.033045
Journal volume & issue
Vol. 1, no. 3
p. 033045

Abstract

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We report on a chiral observable upon ionization of a chiral molecule (methyloxirane) by a strong elliptically polarized laser field: a rotation of the photoelectron momentum distribution, which is enantiosensitive and forward/backward asymmetric. We explain this forward/backward asymmetric rotation of the count maxima to be equivalent to a dependence of the photoelectron circular dichroism on the electron emission angle in the plane of polarization.