Radial and Angular Electron Ejection Patterns of Two-Electron Quantum Dots in THz Fields

Abstract

In this work, we develop and apply an ab-initio method to calculate the joint radial- and- angular electron distributions following the interaction of two-electron spherical quantum dots (QD) with intense terahertz pulses of subpicosecond duration. By applying the method to two QDs of different size, we could investigate two particular ionization mechanisms: the direct and the sequential two-photon double ionization. According to our results, the two ionization mechanisms show some similarity in the angular distribution patterns, whereas the corresponding radial distributions are distinctly different, associated with their joint kinetic energy spectrum. We also discuss the time-evolution of the ionization process in the context of the different nature of the interaction of the QD with the external radiation and the electron–electron correlation interactions.

Keywords

• ab-initio
• multiphoton ionisation
• radial distributions
• angular distributions
• configuration interaction