Designing covalent organic frameworks with Co-O4 atomic sites for efficient CO2 photoreduction

Qian Zhang; Shuaiqi Gao; Yingying Guo; Huiyong Wang; Jishi Wei; Xiaofang Su; Hucheng Zhang; Zhimin Liu; Jianji Wang

doi:10.1038/s41467-023-36779-4

Nature Communications (Feb 2023)

Designing covalent organic frameworks with Co-O4 atomic sites for efficient CO2 photoreduction

Qian Zhang,
Shuaiqi Gao,
Yingying Guo,
Huiyong Wang,
Jishi Wei,
Xiaofang Su,
Hucheng Zhang,
Zhimin Liu,
Jianji Wang

Affiliations

Qian Zhang: Key Laboratory of Green Chemical Media and Reactions (Ministry of Education), Collaborative Innovation Centre of Henan Province for Green Manufacturing of Fine Chemicals, School of Chemistry and Chemical Engineering, Henan Normal University
Shuaiqi Gao: Key Laboratory of Green Chemical Media and Reactions (Ministry of Education), Collaborative Innovation Centre of Henan Province for Green Manufacturing of Fine Chemicals, School of Chemistry and Chemical Engineering, Henan Normal University
Yingying Guo: Key Laboratory of Green Chemical Media and Reactions (Ministry of Education), Collaborative Innovation Centre of Henan Province for Green Manufacturing of Fine Chemicals, School of Chemistry and Chemical Engineering, Henan Normal University
Huiyong Wang: Key Laboratory of Green Chemical Media and Reactions (Ministry of Education), Collaborative Innovation Centre of Henan Province for Green Manufacturing of Fine Chemicals, School of Chemistry and Chemical Engineering, Henan Normal University
Jishi Wei: Department of Electrical and Computer Engineering, National University of Singapore
Xiaofang Su: Key Laboratory of Green Chemical Media and Reactions (Ministry of Education), Collaborative Innovation Centre of Henan Province for Green Manufacturing of Fine Chemicals, School of Chemistry and Chemical Engineering, Henan Normal University
Hucheng Zhang: Key Laboratory of Green Chemical Media and Reactions (Ministry of Education), Collaborative Innovation Centre of Henan Province for Green Manufacturing of Fine Chemicals, School of Chemistry and Chemical Engineering, Henan Normal University
Zhimin Liu: Beijing National Laboratory for Molecular Sciences, Key Laboratory of Colloid, Interface and Thermodynamics, CAS Research/Education Centre for Excellence in Molecular Sciences, Institute of Chemistry, Chinese Academy of Sciences
Jianji Wang: Key Laboratory of Green Chemical Media and Reactions (Ministry of Education), Collaborative Innovation Centre of Henan Province for Green Manufacturing of Fine Chemicals, School of Chemistry and Chemical Engineering, Henan Normal University

DOI: https://doi.org/10.1038/s41467-023-36779-4
Journal volume & issue: Vol. 14, no. 1
pp. 1 – 11

Abstract

Read online

A class of inexpensive aminoanthraquinone organic dyes are shown to facilitate visible-light-driven CO2 reduction. Overall reaction efficiencies were found to be optimal when both electron donating and accepting groups were on a single dye molecule.

Published in Nature Communications

ISSN: 2041-1723 (Online)
Publisher: Nature Portfolio
Country of publisher: United Kingdom
LCC subjects: Science
Website: https://www.nature.com/ncomms/

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