Instant and delayed effects of March biomass burning aerosols over the Indochina Peninsula

Abstract

By analyzing observations and simulations from the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem), we investigated instant and delayed responses of large-scale atmospheric circulations and precipitation to biomass burning (BB) aerosols over the Indochina Peninsula (ICP) in the peak emission of March. The results show that the BB aerosols inhibit precipitation over the ICP in March and promote precipitation from early April to mid April. Specifically, the March BB aerosols over the ICP can induce mid- to lower-tropospheric heating and planetary boundary layer cooling to enhance local atmospheric stability; meanwhile, the perturbation heating can trigger an anomalous low in the lower troposphere to moisten the mid troposphere. However, the convection suppression due to the stabilized atmosphere dominates over the favorable water-vapor condition induced by large-scale circulation responses, leading to overall reduced precipitation over the ICP in March. For the delayed effect, the anomalous low can provide more water vapor as the monsoon advances in early April, although it becomes much weaker without BB aerosols' strong heating. On the other hand, the convective instability above 850 hPa is enhanced by more water vapor, resulting in enhanced precipitation over the ICP, northern South China Sea, and southern China. Thereafter, the condensational latent heating gradually takes over from the BB aerosol radiative heating, acting as the main driver for maintaining the anomalous circulation and thus the delayed effect in mid April.