Nature Communications (Apr 2021)

Ordered clustering of single atomic Te vacancies in atomically thin PtTe2 promotes hydrogen evolution catalysis

  • Xinzhe Li,
  • Yiyun Fang,
  • Jun Wang,
  • Hanyan Fang,
  • Shibo Xi,
  • Xiaoxu Zhao,
  • Danyun Xu,
  • Haomin Xu,
  • Wei Yu,
  • Xiao Hai,
  • Cheng Chen,
  • Chuanhao Yao,
  • Hua Bing Tao,
  • Alexander G. R. Howe,
  • Stephen J. Pennycook,
  • Bin Liu,
  • Jiong Lu,
  • Chenliang Su

DOI
https://doi.org/10.1038/s41467-021-22681-4
Journal volume & issue
Vol. 12, no. 1
pp. 1 – 9

Abstract

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Precisely regulating Pt catalytic sites is important and challenging. Herein the authors engineer the clustering of single atomic Te vacancies in atomically thin PtTe2 to optimize the electronic structure, adsorption energy, and catalytic performance of atomically defined Pt sites.