Nature Communications (Apr 2021)
Ordered clustering of single atomic Te vacancies in atomically thin PtTe2 promotes hydrogen evolution catalysis
- Xinzhe Li,
- Yiyun Fang,
- Jun Wang,
- Hanyan Fang,
- Shibo Xi,
- Xiaoxu Zhao,
- Danyun Xu,
- Haomin Xu,
- Wei Yu,
- Xiao Hai,
- Cheng Chen,
- Chuanhao Yao,
- Hua Bing Tao,
- Alexander G. R. Howe,
- Stephen J. Pennycook,
- Bin Liu,
- Jiong Lu,
- Chenliang Su
Affiliations
- Xinzhe Li
- SZU-NUS Collaborative Center and International Collaborative Laboratory of 2D Materials for Optoelectronic Science and Technology of Ministry of Education, Institute of Microscale Optoelectronics, Shenzhen University
- Yiyun Fang
- SZU-NUS Collaborative Center and International Collaborative Laboratory of 2D Materials for Optoelectronic Science and Technology of Ministry of Education, Institute of Microscale Optoelectronics, Shenzhen University
- Jun Wang
- SZU-NUS Collaborative Center and International Collaborative Laboratory of 2D Materials for Optoelectronic Science and Technology of Ministry of Education, Institute of Microscale Optoelectronics, Shenzhen University
- Hanyan Fang
- Department of Chemistry, National University of Singapore
- Shibo Xi
- Institute of Chemical and Engineering Sciences, Agency for Science, Technology and Research (A*STAR)
- Xiaoxu Zhao
- Department of Materials Science and Engineering, National University of Singapore
- Danyun Xu
- SZU-NUS Collaborative Center and International Collaborative Laboratory of 2D Materials for Optoelectronic Science and Technology of Ministry of Education, Institute of Microscale Optoelectronics, Shenzhen University
- Haomin Xu
- Department of Chemistry, National University of Singapore
- Wei Yu
- Department of Chemistry, National University of Singapore
- Xiao Hai
- Department of Chemistry, National University of Singapore
- Cheng Chen
- Department of Chemistry, National University of Singapore
- Chuanhao Yao
- Department of Chemistry, National University of Singapore
- Hua Bing Tao
- School of Chemical and Biomedical Engineering, Nanyang Technological University
- Alexander G. R. Howe
- Department of Materials Science and Engineering, National University of Singapore
- Stephen J. Pennycook
- Department of Materials Science and Engineering, National University of Singapore
- Bin Liu
- School of Chemical and Biomedical Engineering, Nanyang Technological University
- Jiong Lu
- Department of Chemistry, National University of Singapore
- Chenliang Su
- SZU-NUS Collaborative Center and International Collaborative Laboratory of 2D Materials for Optoelectronic Science and Technology of Ministry of Education, Institute of Microscale Optoelectronics, Shenzhen University
- DOI
- https://doi.org/10.1038/s41467-021-22681-4
- Journal volume & issue
-
Vol. 12,
no. 1
pp. 1 – 9
Abstract
Precisely regulating Pt catalytic sites is important and challenging. Herein the authors engineer the clustering of single atomic Te vacancies in atomically thin PtTe2 to optimize the electronic structure, adsorption energy, and catalytic performance of atomically defined Pt sites.