Physical Review Research (Jul 2023)

Tilted spirals and low-temperature skyrmions in Cu_{2}OSeO_{3}

  • M. Crisanti,
  • A. O. Leonov,
  • R. Cubitt,
  • A. Labh,
  • H. Wilhelm,
  • Marcus P. Schmidt,
  • C. Pappas

DOI
https://doi.org/10.1103/PhysRevResearch.5.033033
Journal volume & issue
Vol. 5, no. 3
p. 033033

Abstract

Read online Read online

The bulk helimagnet Cu_{2}OSeO_{3} represents a unique example in the family of B20 cubic helimagnets exhibiting a tilted spiral and skyrmion phase at low temperatures when the magnetic field is applied along the easy 〈001〉 crystallographic direction. Here we present a systematic study of the stability and ordering of these low-temperature magnetic states. We focus our attention on the temperature and field dependencies of the tilted spiral state that we observe persisting up to above T=35 K, i.e., up to higher temperatures than reported so far. We discuss these results in the frame of the phenomenological theory introduced by Dzyaloshinskii in an attempt to reach a quantitative description of the experimental findings. We find that the anisotropy constants, which are the drivers behind the observed behavior, exhibit a pronounced temperature dependence. This explains the differences in the behavior observed at high temperatures (above T=18 K), where the cubic anisotropy is weak, and at low temperatures (below T=18 K), where a strong cubic anisotropy induces an abrupt appearance of the tilted spirals out of the conical state and enhances the stability of skyrmions.