Experimental Study on Hydrogen Recombination Characteristics of a Passive Autocatalytic Recombiner during Spray Operation

Abstract

During an accident, hydrogen distribution in a containment building of a nuclear power plant (NPP) and characteristics of hydrogen depletion by passive autocatalytic recombiners (PARs) differ depending on the thermal-hydraulic behaviors occurring in the containment. A spray system installed in the NPP containment to control the pressure in accident conditions may interact with PAR operations. This study intended to experimentally evaluate the hydrogen removal characteristics of a grid-type PAR when a spray was operating. For the experimental simulation of hydrogen recombination characteristics of the PAR affected by a spray operation, we used the SPARC experimental facility, which was equipped with a pressure vessel capable of controlling the wall temperature with a volume of 82 m3. To measure gas species concentrations, 14 probes each for hydrogen, oxygen, and water vapor were installed. Two tests were designed depending on the spray initiation time. The SSP3 test was an experiment to simulate an accident in which the PAR operated as hydrogen was released after the spray is activated, and the SSP4 test was an experiment to simulate an accident in which the spray began after the operation of the PAR was initiated by the hydrogen release. In the experiment, two contradictory results were obtained, which were an increased start-up delay time of the PAR by early initiation of the spray and a negligible impact on the PAR’s performance by the delayed initiation of the spray.

Keywords

• hydrogen mitigation
• passive autocatalytic recombiner
• nuclear power plant
• fuel cladding oxidation
• hydrogen generation
• spray