New Journal of Physics (Jan 2013)

Measurement of optical second-harmonic generation from an individual single-walled carbon nanotube

  • M J Huttunen,
  • O Herranen,
  • A Johansson,
  • H Jiang,
  • P R Mudimela,
  • P Myllyperkiö,
  • G Bautista,
  • A G Nasibulin,
  • E I Kauppinen,
  • M Ahlskog,
  • M Kauranen,
  • M Pettersson

DOI
https://doi.org/10.1088/1367-2630/15/8/083043
Journal volume & issue
Vol. 15, no. 8
p. 083043

Abstract

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We show that optical second-harmonic generation (SHG) can be observed from individual single-walled carbon nanotubes (SWCNTs) and, furthermore, allows imaging of individual tubes. Detailed analysis of our results suggests that the structural non-centrosymmetry, as required for SHG, arises from the non-zero chiral angle of the SWCNT. SHG thus has potential as a fast, non-destructive and simple method for imaging of individual nanomolecules and for probing their chiral properties.