New Journal of Physics (Jan 2012)

Ultrafast dynamics and phonon softening in Fe1+ySe1−xTex single crystals

  • C W Luo,
  • I H Wu,
  • P C Cheng,
  • J-Y Lin,
  • K H Wu,
  • T M Uen,
  • J Y Juang,
  • T Kobayashi,
  • Y C Wen,
  • T W Huang,
  • K W Yeh,
  • M K Wu,
  • D A Chareev,
  • O S Volkova,
  • A N Vasiliev

DOI
https://doi.org/10.1088/1367-2630/14/10/103053
Journal volume & issue
Vol. 14, no. 10
p. 103053

Abstract

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The ultrafast quasiparticle dynamics of Fe _1+ _y Se _1− _x Te _x single crystals were investigated by dual-color transient reflectivity measurements (Δ R / R ) from 4.3 to 290 K. The electron–phonon coupling strength λ (=0.16–0.01) and the temperature-dependent energy of longitudinal-acoustic phonons were, respectively, obtained from the relaxation time of a fast component and the period of an oscillation component in Δ R / R . Such a small λ demonstrates the unconventional origin of superconductivity in FeSe. Moreover, the temperature-dependent Δ R / R exhibits anomalous changes at T _c , 90 K and 230 K, unambiguously revealing the phase transition as well as the phonon softening via the magnetoelastic effect.